超低有质动力势能场中原子强场双电离机制研究
Study on Double Ionization Mechanism of Atom in Ultra-Low Ponderomotive Potential Field
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摘要: 利用三维经典系综模型, 研究了超低有质动力势能场下碱土金属原子的强场双电离机制, 并比较了较高有质动力势能场的情况。结果显示, 较高有质动力势能场下, 双电离过程仍然可以用三步再碰撞机制来解释。然而, 超低有质动力势能场下, 双电离过程显示出较新颖的特性, 比如双电离产率随原子电离能的增大而增大, 这很难用再碰撞机制来解释。反演分析两电子的经典轨迹表明, 超低有质动力势能场中, 两电子脱离母核离子的束缚之前, 在核的有效区域内发生了“缩小版回碰”; 然后, 处于较高激发态的电子在激光场的作用下先电离; 处于超低激发态的电子则往往需要多次往返母核离子, 从而从激光场中获得足够的能量而电离, 这与三步再碰撞机制明显不同。进一步研究表明, 在超低激光强度且波长较短时, “缩小版回碰”起主导作用, 当波长较长时再碰撞机制起主导作用。Abstract: By a three-dimensional classical ensemble method, double ionization mechanism of alkaline-earth metal atoms by ultra-low ponderomotive potential fields was investigated, and the higher ponderomotive potential field is compared. The results show that the double ionization process can still be explained by the three-step recolision mechanism at a higher ponderomotive potential fields. However, under the ultra-low ponderomotive potential fields, the double ionization process shows interesting phenomenon. For example, the double ionization yield increases with the increase of atomic ionization energy, which is difficult to be understood by the recollisional mechanism. The trajectory back analysis show that, the collision process takes place in the effective region of the nucleus at ultra-low ponderomotive potential fields, which is called "miniature recollision". Then, the first electron is ionized by the laser field. The second electron usually needs to return to the nucleus several times, and absorb enough energy from the laser field to be ionized. Further sdudies show that "miniature recollision" mechanism plays a dominant role in double ionization at shorter wavelengths, and the recollision mechanism is dominant at longer wavelengths.